83 Search Results

Here, we report the first evidence of spin interference in exclusive 𝐽/𝜓 → 𝑒⁺⁢𝑒⁻ photoproduction in ultraperipheral heavy-ion collisions at STAR at $$\sqrt{𝑠_{𝑁⁢𝑁}}$$ = 200  GeV. In Au + Au collisions, a negative cos⁡(2⁢𝜙) modulation is found for 𝑝_𝑇 < 120  MeV/𝑐 with a significance of 3.2⁢𝜎, while the isobar data (Ru + Ru, Zr + Zr) show a consistent negative modulation with a significance of 1.9⁢𝜎, opposite in sign to that in 𝜌⁰ → 𝜋⁺⁢𝜋⁻ photoproduction. This establishes for the first time that the interference sign is controlled by the spin structure of the final-state daughters, resolving the ambiguity present inmore » the all-boson 𝜌⁰ channel. The compact 𝐽/𝜓 probes gluon distributions at perturbative scales, resulting in a weaker modulation and providing stringent constraints on color glass condensate calculations. These findings demonstrate that spin-dependent interference in heavy vector mesons provides a new, experimentally accessible handle on gluon structure beyond traditional cross-section measurements.« less

Correlated oxides such as VO₂ exhibit an electrically driven insulator–metal transition (IMT) that underlies their promise for neuromorphic and memory devices. Yet the IMT is not a uniform bulk process but a spatiotemporal phenomenon in which local heating nucleates filaments, contracts or dissolves them with the electric field, and couples to the environment. In this work, we directly image the VO₂ IMT dynamics by mid-wave infrared, thermography synchronized with electrical transport, resolving device temperature with micrometer spatial and microsecond temporal resolution. At the single-device level, we capture the full cycle of filament nucleation, contraction, and relaxation during current/voltage-driven resistive switching.more » At the array level, we show that heat propagates across etched gaps with an effective length scale of ∼131 µm, enabling cooperative behaviors among electrically isolated devices. Short-range distanced devices exhibit mutual filament attraction and sequential dissolution, while long-range distanced devices differentiate into distinct roles: drivers that initiate switching, cooperative responders that undergo assisted self-oscillations, and passive reporters that record the thermal field. Furthermore, these results reframe thermal crosstalk, long regarded as parasitic, as an intrinsic coupling channel and design principle for organizing collective switching behaviors, with direct implications for emergent circuit functionality in neuromorphic and unconventional computing architectures.« less

Chiral molecules, ubiquitous in chemistry and biology, can differentiate electrons by their spin, a phenomenon known as chirality-induced spin selectivity (CISS). Despite its robustness and technological relevance, CISS has resisted conventional explanation: Spin-orbit coupling (SOC) models cannot fully account for the observed magnitude, room-temperature persistence, or equilibrium signatures. Here, we argue that structural chirality enforces a twin-pair exchange mechanism via the indistinguishability principle, which intrinsically couples spin and spatial degrees of freedom such that wave functions cannot be factorized into spin and spatial components. We derive an effective Hamiltonian that describes both transport and equilibrium CISS phenomena and is non-Hermitian.more » However, the inherent pseudo-Hermiticity, with $$\mathscr{PT}$$ symmetry as a special case, ensures real eigenvalues and thermodynamic consistency. We demonstrate that our framework is a step toward resolving long-standing anomalies of CISS. It situates CISS alongside equilibrium symmetry-breaking phenomena such as ferromagnetism and superconductivity, with implications for spintronics, catalysis, and the origins of biological homochirality.« less

Land-atmosphere interactions play a critical role in the evolution and formation of low-level clouds. The different states of coupling between low-level clouds and the surface are uncertain, primarily over continental regions, where complex thermodynamics complicates their investigation. This study uses observations from the Atmospheric Radiation Measurement User Facility to explore cloud-surface coupling and perform a climatological analysis of this interaction in five countries across three continents. The results reveal consistent coupling thresholds and average percentages across the five sites, with coupled clouds accounting for 66% of the cases and decoupled clouds for 34%. Thermodynamic and dynamic evaluations show distinct differencesmore » between coupled and decoupled clouds. Coupled clouds are characterized by humid environments, in which vertical motions connect the surface and lower atmosphere to the cloud base, conditions that favor the formation of boundary layer clouds. Decoupled clouds prefer to occur in a drier and colder environment with vertical motions inside the boundary layer being detached from the cloud base, under which boundary layer clouds are hard to form. Coupled clouds peak during warmer hours and seasons, and vice versa for decoupled clouds. This study underscores the complexity of cloud-land-surface interactions and paves the way for further investigations into cloud formation and evolution under different atmospheric environments.« less

The STAR experiment reports new, high-precision measurements of the transverse single-spin asymmetries for 𝜋^± within jets, namely the Collins asymmetries, from transversely polarized 𝑝^↑⁢𝑝 collisions at $$\sqrt{s}$$ = 510 GeV. The energy-scaled distribution of jet transverse momentum, 𝑥_T = 2⁢𝑝_T,jet/$$\sqrt{s}$$, shows a remarkable consistency for Collins asymmetries of 𝜋^± in jets between $$\sqrt{s}$$ = 200 GeV and 510 GeV. This indicates that the Collins asymmetries are nearly energy independent, with, at most, a very weak scale dependence in 𝑝^↑⁢𝑝 collisions. These results extend to high-momentum scales (𝑄² ≤ 3400 GeV²) and enable unique tests of evolution and universality in themore » transverse-momentum-dependent formalism, thus providing important constraints for the Collins fragmentation functions.« less

The conservation of lepton flavor is a prediction of the Standard Model and is still an excellent approximate symmetry despite our observation of neutrino oscillations. Lepton flavor violation by one or two units has been discussed for decades, with several dedicated experiments exploring the vast model landscape but no discoveries so far. Here, we explore operators and processes that violate at least one lepton flavor by three units and identify testable signatures. In the Standard Model effective field theory, such operators already arise at mass dimension 7 and can be tested through their contributions to Michel parameters in leptonic decays.more » True neutrinoless charged-lepton flavor violation arises at mass dimension 10 and can realistically only be seen in the tau decay channels 𝜏 → $$𝑒⁢𝑒⁢𝑒⁢\bar{𝜇}⁢\bar{𝜇}$$ or 𝜏 → $$𝜇⁢𝜇⁢𝜇\bar{𝑒}\bar{𝑒}$$, for example in Belle II. Testable rates for these tau decays require light new particles and subsequently predict an avalanche of remarkably clean but so-far unconstrained collider signatures.« less

Flavin-based electron bifurcation (FBEB) is employed by microorganisms for controlling pools of redox equivalents by reversibly splitting electron pairs into high- and low-energy levels from an initial midpoint potential. Our ability to harness this phenomenon is crucial for biocatalytic design which is limited by our understanding of energy coupling in the bifurcation system. In Pyrococcus furiosus, FBEB is carried out by the NADH-dependent ferredoxin:NADP+-oxidoreductase (NfnSL), coupling the uphill reduction of ferredoxin in NfnL to the downhill reduction of NAD+ in NfnS from oxidation of NADPH. Flanking the bifurcating flavin are two site-differentiated iron-sulfur clusters; the nearest is a glutamate-ligated [4Fe-4S]more » cluster in NfnL. Recent biochemical experiments substituting the native glutamate with cysteine led to loss of coupling between the uphill and downhill pathways, in contrast to the tight thermodynamic coupling in the native system. To understand how this decoupling is biochemically manifested by the cysteine-substituted [4Fe-4S] in NfnL, we employed electron paramagnetic resonance (EPR) spectroscopy to identify changes in electronic architecture and square wave voltammetry (SWV) to probe thermodynamic shifts produced by the substitution. We observed notable g-value shifts in the EPR for the cysteine-substituted iron-sulfur cluster in addition to significant downward shifts in the redox potential, as well as the disappearance of several low-field signals observed in the native NfnSL complex. These results suggest the site-differentiated glutamate residue facilitates higher spin states in the [4Fesingle bond4S] cluster to bridge energetic gaps in electron transfer to the bifurcating flavin in the native complex, preventing unwanted short-circuiting seen in the cysteine-substituted complex.« less

The hadron physics community has been actively debating the interpretation of so-called mechanical properties of hadrons. Nonrelativistic quantum-mechanical systems like the hydrogen atom have been appealed to in these debates as analogies. Since such appeals are likely to continue, it is important to have Galilei-covariant expressions for matrix elements of the energy-momentum tensor. In this work, I obtain Galilei-covariant breakdowns of such matrix elements into mechanical form factors, with a special focus on spin-half states. I additionally study the spatial densities associated with these form factors, using the pilot wave interpretation to guide their breakdown into contributions from internal structuremore » and from quantum-mechanical effects such as wave packet dispersion. For completeness, I also obtain nonrelativistic Breit frame densities.« less

PdAu/SiO₂ catalysts were synthesized by strong electrostatic adsorption (SEA) and characterized by TEM, DRIFTS, XRD, XAS, and O₂-TPD. The use of group 1 alkali salt solutions to control pH during SEA syntheses led to uptake of alkali metals observed reductions in the densities of terminal silanol groups of the SiO₂ support. In the absence of alkali metals, PdAu/SiO₂ catalyzes oxidative C-N bond formation between methanol and dimethylamine (DMA), yielding dimethylformamide (DMF) with ∼95 % carbon selectivity (CO₂ ∼5 %) at temperatures below 413 K. When Na, K, and Cs were present on the catalyst, methyl formate (MF) and tetramethylurea (TMU)more » were observed as additional products (combined ∼30 % carbon selectivity) while only TMU was detected for the Li-promoted catalyst. Total coupling product rate increased for promoted samples in the order Li < Na < Cs < K, and the apparent kinetics over the Cs-promoted catalyst were distinct from those over the alkali-free catalyst as the apparent reaction order with respect to DMA decreased and the apparent activation energy increased. Finally, this work demonstrates the sensitivity of oxidative coupling reactions to alkali metal promoters and the opportunity to achieve alkali promotion of metal catalysts during SEA synthesis.« less

Combining the synthetic tunability of molecular compounds with the optical selection rules of transition metal dichalcogenides (TMDCs) that derive from spin-valley coupling could provide interesting opportunities for the readout of quantum information. However, little is known about the electronic and spin interactions at such interfaces and the influence on spin-valley relaxation. Here, in this work, vanadyl phthalocyanine (VOPc) molecular layers are thermally evaporated on WSe₂ to explore the effect of molecular layer thickness on excited-state spin-valley polarization. The thinnest molecular layer supports an interfacial state which destroys the spin-valley polarization almost instantaneously, whereas a thicker molecular layer results in longer-livedmore » spin-valley polarization than the WSe₂ monolayer alone. The mechanism appears to involve a tightly bound species at the molecule/TMDC interface that strengthens exchange interactions and is largely avoided in thicker VOPc layers that isolate electrons from WSe₂ holes.« less